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Dehydrogenative coupling to enable the enantioselective total synthesis of (-)-simaomicin α

Yizhong Wang; Chao Wang; John R. Butler; Joseph M. Ready

(Profiled Author: Joseph M Ready)

Angewandte Chemie - International Edition. 2013;52(41):10796-10799.

Abstract

The anticancer natural product simaomicin α has been synthesized. Asymmetric synthesis allowed the assignment of absolute stereochemistry. The enantiomer of the naturally occurring substance shows potent cytotoxicity towards Gram-positive bacteria and human cancer cells. Bn=benzyl, BOM=benzyloxymethyl. Copyright © 2013 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

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